Gandara-Loe, Jesus; Zhang, Qi; Jose Villora-Pico, Juan; Sepulveda-Escribano, Antonio; Pastor-Perez, Laura; Ramirez Reina, Tomas;
Reverse water gas shift (RWGS) competes with methanation as a direct pathway in the CO2 recycling route, with methanation being a dominant process in the low-temperature window and RWGS at higher temperatures. This work showcases the design of multi-component catalysts for a full-temperature-range RWGS behavior by suppressing the methanation reacti...
Sun, Taolue Wu, Zhenyu Wang, Gang Li, Zengxi Li, Chunshan Wang, Emiang
A series of Ni/gamma-Al2O3 and Ni-Mo/gamma-Al2O3 catalysts were prepared and evaluated for the hydrogenation of methyl acrylate to methyl propionate in a fixed-bed reactor. Physicochemical characterizations of these catalysts were carried out with Brunauer-Emmett-Teller analysis, X-ray diffraction, UV-vis diffuse reflectance spectroscopy, Raman spe...
Sun, Taolue Wu, Zhenyu Wang, Gang Li, Zengxi Li, Chunshan Wang, Erqiang
A series of Ni/gamma-Al2O3 and Ni-Mo/gamma-Al2O3 catalysts were prepared and evaluated for the hydrogenation of methyl acrylate to methyl propionate in a fixed-bed reactor. Physicochemical characterizations of these catalysts were carried out with Brunauer-Emmett-Teller analysis, X-ray diffraction, UV-vis diffuse reflectance spectroscopy, Raman spe...
Sun, Taolue Wu, Zhenyu Wang, Gang Li, Zengxi Li, Chunshan Wang, Erqiang
A series of Ni/gamma-Al2O3 and Ni-Mo/gamma-Al2O3 catalysts were prepared and evaluated for the hydrogenation of methyl acrylate to methyl propionate in a fixed-bed reactor. Physicochemical characterizations of these catalysts were carried out with Brunauer-Emmett-Teller analysis, X-ray diffraction, UV-vis diffuse reflectance spectroscopy, Raman spe...
Yue, Xia Chen, Dezhen Luo, Jia Huang, Zhen Hong, Liu Hu, Yuyan
Thermochemical conversion of biomass into methane is a promising way for bioenergy recovery and alleviate natural gas shortage; however, the available technologies are queried by the complex procedures. This paper proposed a new approach for the direct synthesis of methane-rich gases from reed pyrolysis volatile at atmospheric pressure, according t...
Yue, Xia Chen, Dezhen Luo, Jia Huang, Zhen Hong, Liu Hu, Yuyan
Thermochemical conversion of biomass into methane is a promising way for bioenergy recovery and alleviate natural gas shortage; however, the available technologies are queried by the complex procedures. This paper proposed a new approach for the direct synthesis of methane-rich gases from reed pyrolysis volatile at atmospheric pressure, according t...
Yue, Xia Chen, Dezhen Luo, Jia Huang, Zhen Hong, Liu Hu, Yuyan
Thermochemical conversion of biomass into methane is a promising way for bioenergy recovery and alleviate natural gas shortage; however, the available technologies are queried by the complex procedures. This paper proposed a new approach for the direct synthesis of methane-rich gases from reed pyrolysis volatile at atmospheric pressure, according t...
He, Feng Zhuang, Jiahao Lu, Bin Liu, Xianglin Zhang, Jianling Gu, Fangna Zhu, Minghui Xu, Jing Zhong, Ziyi Xu, Guangwen
...
Developing Ni-based catalysts with high activity and stability in low-temperature methanation is necessary due to their sintering and coking at high temperatures. Here, we report our developed novel Ni-Zr-Al catalysts derived from Ni-Zr-Al ternary hydrotalcites synthesized by a hydrothermal process, followed by a reduction in hydrogen. Comparing wi...
He, Feng Zhuang, Jiahao Lu, Bin Liu, Xianglin Zhang, Jianling Gu, Fangna Zhu, Minghui Xu, Jing Zhong, Ziyi Xu, Guangwen
...
Developing Ni-based catalysts with high activity and stability in low-temperature methanation is necessary due to their sintering and coking at high temperatures. Here, we report our developed novel Ni-Zr-Al catalysts derived from Ni-Zr-Al ternary hydrotalcites synthesized by a hydrothermal process, followed by a reduction in hydrogen. Comparing wi...
Xu, Bin Xie, Jianjun Zhan, Hao Yin, Xiuli Wu, Chuangzhi Liu, Hao
In this study, a packed-bed dielectric barrier discharge (DBD) reactor was developed to investigate the removal of biomass tar in a fuel gas atmosphere. Toluene was used as the tar surrogate, and the catalyst used was a Nickel-based catalyst (Ni/gamma-Al2O3) because of its high activity and low cost. In addition, another two kinds of packing materi...