Zhang, Tengfei Wang, Weiwei Gu, Fangna Xu, Wenqing Zhang, Jianling Li, Zhenxing Zhu, Tingyu Xu, Guangwen Zhong, Ziyi Su, Fabing
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This work reports a strategy to promote the low-temperature CO2 methanation on the Ni-based catalyst by tuning the surface oxygen vacancy and medium-strength basic sites of the CeO2 support and thus changing the reaction pathway. La species was introduced into CeO2 support and calcined at 600 degrees C (CeO2-La-600) to form a La-Ce-O solid solution...
Zhang, Tengfei Wang, Weiwei Gu, Fangna Xu, Wenqing Zhang, Jianling Li, Zhenxing Zhu, Tingyu Xu, Guangwen Zhong, Ziyi Su, Fabing
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This work reports a strategy to promote the low-temperature CO2 methanation on the Ni-based catalyst by tuning the surface oxygen vacancy and medium-strength basic sites of the CeO2 support and thus changing the reaction pathway. La species was introduced into CeO2 support and calcined at 600 degrees C (CeO2-La-600) to form a La-Ce-O solid solution...
Ma, Yuan Liu, Jiao Chu, Mo Yue, Junrong Cui, Yanbin Xu, Guangwen
CeO2 nanorods (CeO2-nrs), CeO2 nanocubes (CeO2-ncs) and CeO2 nanopolyhedrons (CeO2-nps) were prepared by hydrothermal method and then NiO crystallites were deposited on these supports by precipitation-deposition, respectively. The physicchemical properties of Ni/CeO2 catalysts were characterized and performances for carbon dioxide methanation react...
Ma, Yuan Liu, Jiao Chu, Mo Yue, Junrong Cui, Yanbin Xu, Guangwen
CeO2 nanorods (CeO2-nrs), CeO2 nanocubes (CeO2-ncs) and CeO2 nanopolyhedrons (CeO2-nps) were prepared by hydrothermal method and then NiO crystallites were deposited on these supports by precipitation-deposition, respectively. The physicchemical properties of Ni/CeO2 catalysts were characterized and performances for carbon dioxide methanation react...
Guo, Xinpeng Gao, Denglei He, Hongyan Traitangwong, Atsadang Gong, Maoming Meeyoo, Vissanu Peng, Zhijian Li, Chunshan
The CO2 methanation is an effective strategy for making full use of waste gases and converting them into valuable chemicals. Nowadays, the key challenge is the design of efficient catalysts to enhance low-temperature catalytic performance. A series of hydrotalcite-derived catalysts with tunable metal species were prepared by hydrothermal synthesis ...
Guo, Xinpeng Gao, Denglei He, Hongyan Traitangwong, Atsadang Gong, Maoming Meeyoo, Vissanu Peng, Zhijian Li, Chunshan
The CO2 methanation is an effective strategy for making full use of waste gases and converting them into valuable chemicals. Nowadays, the key challenge is the design of efficient catalysts to enhance low-temperature catalytic performance. A series of hydrotalcite-derived catalysts with tunable metal species were prepared by hydrothermal synthesis ...
Ma, Yuan Liu, Jiao Chu, Mo Yue, Junrong Cui, Yanbin Xu, Guangwen
The key challenge for CO2 methanation, an eight-electron process under kinetic limitation, relies on the design of non-noble metal catalysts so as to achieve high activity at low reaction temperatures. In this work, four Ni-based catalysts with different supports were prepared and tested for CO2 methanation at 250-550 degrees C in a fixed bed quart...
Ma, Yuan Liu, Jiao Chu, Mo Yue, Junrong Cui, Yanbin Xu, Guangwen
The key challenge for CO2 methanation, an eight-electron process under kinetic limitation, relies on the design of non-noble metal catalysts so as to achieve high activity at low reaction temperatures. In this work, four Ni-based catalysts with different supports were prepared and tested for CO2 methanation at 250-550 degrees C in a fixed bed quart...
Guo, Xinpeng Peng, Zhijian Hu, Mingxiang Zuo, Cuncun Traitangwong, Atsadang Meeyoo, Vissanu Li, Chunshan Zhang, Suojiang
The Ni nanoparticles supported on Al2O3 metal oxides with different Ni2+/Al3+ molar ratios from 1/1 to 6/1 (denoted as Ni(x)AL-MO) derived from Ni-Al hydrotalcite precursors (NixAl-LDHs) were prepared and applied to CO2 methanation at a low temperature. By adjusting the Ni2+/Al3+ ratios, the alkaline and reducibility of the catalysts were designed,...
Guo, XP Peng, ZJ Hu, MX Zuo, CC Traitangwong, A Meeyoo, V Li, CS Zhang, SJ Guo, Xinpeng Peng, Zhijian
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The Ni nanoparticles supported on Al2O3 metal oxides with different Ni2+/Al3+ molar ratios from 1/1 to 6/1 (denoted as Ni(x)AL-MO) derived from Ni-Al hydrotalcite precursors (NixAl-LDHs) were prepared and applied to CO2 methanation at a low temperature. By adjusting the Ni2+/Al3+ ratios, the alkaline and reducibility of the catalysts were designed,...