The free energy principle made simpler but not too simple
Future UK solar system science
Reaching the fundamental limitation in CO2 reduction to CO with single atom catalysts
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The electrochemical CO2 reduction reaction (CO2RR) to value-added chemicals with renewable electricity is a promising method to decarbonize parts of the chemical industry. Recently, single metal atoms in nitrogen-doped carbon (MNC) have emerged as potential electrocatalysts for CO2RR to CO with high activity and faradaic efficiency, although the re...
Confocal microscopy for in situ multi-modal characterization and patterning of laser-reduced graphene oxide
Graphene oxide (GO) films can be readily prepared at wafer scale, then reduced to form graphene-based conductive circuits relevant to a range of practical device applications. Among a variety of reduction methods, laser processing has emerged as an important technique for localized reduction and patterning of GO films. In this study, the novel use ...
Multigenetic origin of the X-discontinuity below continents: insights from African receiver functions
Constraints on chemical heterogeneities in the upper mantle may be derived from studying the seismically observable impedance contrasts that they produce. Away from subduction zones, several causal mechanisms are possible to explain the intermittently observed X-discontinuity (X) at 230–350 km depth: the coesite-stishovite phase transition, the ens...
Two‐photon polymerization of sugar responsive 4D microstructures
Stimuli-responsive hydrogels have attracted much attention owing to the versatility of their programmed response in offering intelligent solutions for biomimicry applications, such as soft robotics, tissue engineering, and drug delivery. To achieve the complexity of biomimetic structures, two photon polymerization (2PP) has provided a means of fabr...
Modular synthesis of semiconducting graft co-polymers to achieve ‘clickable’ fluorescent nanoparticles with long circula...
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Semiconducting polymer nanoparticles (SPNs) are explored for applications in cancer theranostics because of their high absorption coefficients, photostability, and biocompatibility. However, SPNs are susceptible to aggregation and protein fouling in physiological conditions, which can be detrimental for in vivo applications. Here, a method for achi...
Landau theory-based relaxational modelling of first-order magnetic transition dynamics in magnetocaloric materials
The magnetocaloric effect is often largest within the neighborhood of a first-order phase transition. This effect can be utilized in magnetocaloric refrigeration, which completely eliminates the need for the greenhouse gases utilized in conventional refrigeration. However, such transitions present unique dynamical effects and are accompanied by hys...
Role of electron localisation in H adsorption and hydride formation in the Mg basal plane under aqueous corrosion: a fir...
Understanding hydrogen-metal interactions is important in various fields of surface science, including the aqueous corrosion of metals. The interaction between atomic H and a Mg surface is a key process for the formation of sub-surface Mg hydride, which may play an important role in Mg aqueous corrosion. In the present work, we performed first-prin...
A sprayed graphene transistor platform for rapid and low-cost chemical sensing
We demonstrate a novel and versatile sensing platform, based on electrolyte-gated graphene field-effect transistors, for easy, low-cost and scalable production of chemical sensor test strips. The Lab-on-PCB platform is enabled by low-boiling, low-surface-tension sprayable graphene ink deposited on a substrate manufactured using a commercial printed...
