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Versatile functionalization of carbon electrodes with a polypyridine ligand: metallation and electrocatalytic H+ and CO2 reduction

Authors
Type
Published Article
Volume
51
Issue
14
Pages
2995–2998
Identifiers
DOI: 10.1039/c4cc10027a
Source
USPC - SET - SVS
Keywords
License
Unknown

Abstract

A strategy is proposed for immobilization of homogeneous catalysts whereby a glassy carbon electrode is functionalized by electro-grafting of a ligand, terpyridine. The modified electrode can easily be metallated with cobalt and shows activity towards catalytic proton and CO2 reduction. The metal can be removed and the electrode re-metallated at will.

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