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A Mn-N3 single-atom catalyst embedded in graphitic carbon nitride for efficient CO2 electroreduction

Authors
  • Feng, Jiaqi1, 2
  • Gao, Hongshuai1
  • Zheng, Lirong3
  • Chen, Zhipeng4, 5
  • Zeng, Shaojuan1
  • Jiang, Chongyang1, 2
  • Dong, Haifeng1
  • Liu, Licheng4, 5
  • Zhang, Suojiang1, 2
  • Zhang, Xiangping1, 2, 4
  • 1 Chinese Academy of Sciences, Beijing, 100190, P.R. China , Beijing (China)
  • 2 University of Chinese Academy of Science, Beijing, 100049, P.R. China , Beijing (China)
  • 3 Chinese Academy of Sciences, Beijing, 100049, P.R. China , Beijing (China)
  • 4 Dalian National Laboratory for Clean Energy, Dalian, 116023, P.R. China , Dalian (China)
  • 5 Chinese Academy of Sciences, Qingdao, 266101, P.R. China , Qingdao (China)
Type
Published Article
Journal
Nature Communications
Publisher
Springer Nature
Publication Date
Aug 28, 2020
Volume
11
Issue
1
Identifiers
DOI: 10.1038/s41467-020-18143-y
Source
Springer Nature
License
Green

Abstract

Developing effective catalysts based on earth abundant elements is critical for electrochemical CO2 reduction. Here, the authors prepare a manganese single atom catalyst with high CO2 reduction performance, which can be attributed to the Mn-N3 site embedded in graphitic carbon nitride.

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