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Magnetic field-induced one-magnon Raman scattering in the magnon Bose-Einstein condensation phase of TlCuCl$_{3}$

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Preprint
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DOI: 10.1103/PhysRevB.77.134420
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arXiv
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Abstract

We report the observation of the $A_{\rm g}$-symmetric one-magnon Raman peak in the magnon Bose-Einstein condensation phase of TlCuCl$_{3}$. Its Raman shift traces the one-magnon energy at the magnetic $\Gamma$ point, and its intensity is proportional to the squared transverse magnetization. The appearance of the one-magnon Raman scattering originates from the exchange magnon Raman process and reflects the change of the magnetic-state symmetry. Using the bond-operator representation, we theoretically clarify the Raman selection rules, being consistent with the experimental results.

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