Hydrogenic Rydberg states of molecular van der Waals complexes: resolved Rydberg spectroscopy of DABCO-N2.
- Published Article
Physical review letters
- Publication Date
Jan 30, 2004
The complementary threshold ionization techniques of MATI and ZEKE spectroscopy have been used to reveal well-resolved, long-lived (>10 micros) hydrogenic Rydberg series (50< or =n< or =98) in a van der Waals complex formed between a polyatomic molecule and a diatomic molecule for the first time. The series are observed within 50 cm(-1) of the adiabatic ionization threshold as well as two core-excited thresholds corresponding to excitation of up to two quanta in the van der Waals vibrational mode.
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The corresponding record at NLM can be accessed at https://www.ncbi.nlm.nih.gov/pubmed/14995368