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A detailed account of the measurements of cold collisions in a molecular synchrotron

Authors
  • P. van der Poel, Aernout P.1
  • Bethlem, Hendrick L.1
  • 1 LaserLaB, Department of Physics and Astronomy, Vrije Universiteit, De Boelelaan 1081, Amsterdam, The Netherlands , Amsterdam (Netherlands)
Type
Published Article
Journal
EPJ Techniques and Instrumentation
Publisher
Springer Berlin Heidelberg
Publication Date
Jul 11, 2018
Volume
5
Issue
1
Identifiers
DOI: 10.1140/epjti/s40485-018-0048-y
Source
Springer Nature
Keywords
License
Yellow

Abstract

We have recently demonstrated a general and sensitive method to study low energy collisions that exploits the unique properties of a molecular synchrotron (Van der Poel et al., Phys Rev Lett 120:033402, 2018). In that work, the total cross section for ND3 + Ar collisions was determined from the rate at which ammonia molecules were lost from the synchrotron due to collisions with argon atoms in supersonic beams. This paper provides further details on the experiment. In particular, we derive the model that was used to extract the relative cross section from the loss rate, and present measurements to characterize the spatial and velocity distributions of the stored ammonia molecules and the supersonic argon beams.

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