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Electronic and geometric structure in silver clusters

Authors
Journal
Chemical Physics Letters
0009-2614
Publisher
Elsevier
Publication Date
Volume
192
Issue
1
Identifiers
DOI: 10.1016/0009-2614(92)85439-h
Disciplines
  • Mathematics
  • Physics

Abstract

Abstract One-photon ionization mass spectra were recorded for silver clusters (generated by pulsed laser vaporization) throughout the 4.92 to 5.96 eV energy range. Results include: (i) the observation of electronic structure effects to Ag x , x⩽440 and (ii) the determination of vertical ionization potentials for most x⩽100 and x=138. Data are discussed in terms of various model calculations incorporating particle-size-dependent electronic/geometric structure and compared to analogous measurements of cold sodium and copper clusters.

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