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Fly ash-based geopolymer for Pb removal from aqueous solution

Authors
Journal
Journal of Hazardous Materials
0304-3894
Publisher
Elsevier
Publication Date
Volume
188
Identifiers
DOI: 10.1016/j.jhazmat.2011.01.133
Keywords
  • Adsorption
  • Fly Ash
  • Geopolymer
  • Lead
  • Wastewater Treatment

Abstract

Abstract The aim of this work was to synthesis highly amorphous geopolymer from waste coal fly ash, to be used as an adsorbent for lead Pb(II) removal from aqueous wastewater. The effect of various parameters including geopolymer dosage, initial concentration, contact time, pH and temperature on lead adsorption were investigated. The major components of the used ash in the current study were SiO 2, Al 2O 3 and Fe 2O 3 representing 91.53 wt% of its mass. It was found that the synthesized geopolymer has higher removal capacity for lead ions when compared with that of raw coal fly ash. The removal efficiency increases with increasing geopolymer dosage, contact time, temperature, and the decrease of Pb 2+ initial concentration. The optimum removal efficiency was obtained at pH 5. Adsorption isotherm study indicated that Langmuir isotherm model is the best fit for the experimental data than Freundlich model. It was found also that the adsorption process is endothermic and more favorable at higher temperatures.

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