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Atomically-precise dopant-controlled single cluster catalysis for electrochemical nitrogen reduction

Authors
  • Yao, Chuanhao1, 2
  • Guo, Na3
  • Xi, Shibo4
  • Xu, Cong-Qiao5
  • Liu, Wei1, 6
  • Zhao, Xiaoxu1, 7, 8
  • Li, Jing1
  • Fang, Hanyan1, 6
  • Su, Jie1, 6
  • Chen, Zhongxin1, 7
  • Yan, Huan1
  • Qiu, Zhizhan1, 7
  • Lyu, Pin1
  • Chen, Cheng1, 7
  • Xu, Haomin1, 6
  • Peng, Xinnan1, 6
  • Li, Xinzhe1
  • Liu, Bin9
  • Su, Chenliang10
  • Pennycook, Stephen J.7, 8
  • And 5 more
  • 1 National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore , Singapore (Singapore)
  • 2 Northwestern Polytechnical University (NPU), 127 West Youyi Road, Xi’an, 710072, China , Xi’an (China)
  • 3 National University of Singapore, 2 Science Drive 3, Singapore, 117542, Singapore , Singapore (Singapore)
  • 4 Institute of Chemical and Engineering Sciences, 1 Pesek Road, Jurong Island, 627833, Singapore , Jurong Island (Singapore)
  • 5 Southern University of Science and Technology, Shenzhen, 518055, China , Shenzhen (China)
  • 6 National University of Singapore, Singapore, 117546, Singapore , Singapore (Singapore)
  • 7 NUS Graduate School for Integrative Sciences and Engineering, National University of Singapore, 28 Medical Drive, Singapore, 117456, Singapore , Singapore (Singapore)
  • 8 National University of Singapore, 9 Engineering Drive 1, Singapore, 117575, Singapore , Singapore (Singapore)
  • 9 Nanyang Technological University, Singapore, Singapore , Singapore (Singapore)
  • 10 Shenzhen University, Shenzhen, 518060, China , Shenzhen (China)
  • 11 Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL, 60439, USA , Argonne (United States)
  • 12 Tsinghua University, Beijing, 100084, China , Beijing (China)
  • 13 Brookhaven National Laboratory, Upton, NY, 11973, USA , Upton (United States)
Type
Published Article
Journal
Nature Communications
Publisher
Springer Nature
Publication Date
Sep 01, 2020
Volume
11
Issue
1
Identifiers
DOI: 10.1038/s41467-020-18080-w
Source
Springer Nature
License
Green

Abstract

The fabrication of singly dispersed metal cluster catalysts with atomic-level control of dopants is a long-standing challenge. Here, the authors report a strategy for the synthesis of a precisely doped single cluster catalyst which shows exceptional activity for electrochemical dinitrogen reduction.

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