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Induced contributions in isotropic and anisotropic Rayleigh spectra of fluid H2S

Authors
Journal
Chemical Physics Letters
0009-2614
Publisher
Elsevier
Publication Date
Volume
102
Issue
5
Identifiers
DOI: 10.1016/0009-2614(83)87437-5

Abstract

Abstract Isotropic and anisotropic Rayleigh spectra of fluid H 2S are reported. Collision-induced rotational scattering contributions are considered to explain the spectral features. It is argued that isotropic spectra are mainly due to the dipole-quadrupole polarizability at high frequency while the first hyperpolarizability is significant at low frequency.

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