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Vibrational relaxation of OCS(ν3)

Authors
Journal
Chemical Physics Letters
0009-2614
Publisher
Elsevier
Publication Date
Volume
148
Issue
6
Identifiers
DOI: 10.1016/0009-2614(88)80318-x

Abstract

Abstract A laser-induced fluorescence method has been used to measure rate constants for relaxation of the ν 3 (2062 cm −1) vibrational level of OCS. A frequency-doubled CO 2 laser was used to pump OCS directly to the excited level. At 295 K the rate constants for relaxation by OCS, He, Ar, Kr, H 2, O 2, NO 2 and H 2O were 144, 8.0, 8.0, 8.3, 27, 11, 61 and 675, respectively, in units of 10 −14 cm 3/molecules.

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