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Measurements of exciton–polariton dynamics in ZnO by using nonlinear spectroscopic techniques

Authors
Journal
Journal of Luminescence
0022-2313
Publisher
Elsevier
Publication Date
Volume
112
Identifiers
DOI: 10.1016/j.jlumin.2004.09.033
Keywords
  • Zno
  • Exciton
  • Polariton
  • Four-Wave Mixing

Abstract

Abstract We have studied the exciton–polariton dynamics in a c-face bulk ZnO crystal grown by the seeded vapor transport method. We have performed two-pulse spectrally resolved four-wave mixing (SR-FWM) and three-pulse SR-FWM at T = 10 K. In two-pulse FWM experiment, obtained FWM signals showed the fast dephasing which has been attributed to the strong polariton dispersion of the upper polariton of B exciton. On the other hand, in three-pulse FWM experiment, the signal decay shows the free exciton population relaxation. Observed FWM signal has decayed with time constant ∼ 12 ps which may represent exciton–polariton lifetime.

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